Given the number of atoms of Calcium as 1.204 x 10^24, we can determine the number of moles using the formula:
Number of moles (n) = Number of atoms / Avogadro's number (Nₐ)
n = (1.204 x 10^24 atoms) / (6.022 x 10^23 atoms/mol)
n ≈ 2 moles
Therefore, there are approximately 2 moles in 1.204 x 10^24 atoms of Calcium.