Chang'E-5, China's first lunar sample return mission successfully touched down near the Mons Rumker site (51.8198°W, 43.0570°N) in Oceanus Procellarum on the lunar nearside. The basalt samples collected by Chang'E-5 from the northwest edge of Mons Rümker have significantly enriched our understanding of lunar evolution. Here, a comprehensive record of 72 volcanic eruptions is identified based on the major elements, minerals, and the oxygen three-isotope compositions of Apollo and Chang'E basalt samples from different landing sites and ages; a large composition variation, young eruption ages, and rapid crustal growth of an Imbrian basin (i.e., Imbrium Orientale; ∼3.8 Ga) in the Procellarum area are suggested. Our result implies that the crustal thinning resulting from the South Pole–Aitken basin impact triggered significant upwelling of deep mantle material and contributed to the origin of young basaltic volcanism in western Oceanus Procellarum during the late Imbrian (i.e., ∼3.6–3.8 Ga).